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Development of tritium processing material — A U-Zr alloy as a promising tritium storage material

T. Yamamoto, T. Yoneoka, S. Kokubo, M. Yamawaki1988年Fusion Engineering and DesignIF 1.7出版社

Hydrogen absorption-desorption properties of UZr2.3, 6-phase intermetallic compound, were studied at temperatures ranging from room temperature to 973 K at a hydrogen pressure of 10 to 105 Pa. As a result, separation into ZrH2 and UH3 phases occurred on hydrogenation of UZr2.3. However, the decomposition isotherms of these phases were considerably different from those of the respective pure metals, and this result was attributed to the dissolution of one metal element into the hydride phase of the other metal element. Despite the formation of the UH3 phase, powdering of the alloy specimen on its hydrogenation was remarkably reduced, possibly due to zirconium dissolving into it. Hence, the UZr2.3 is evaluated to be a promising storage material for tritium.

日本語訳

UZr2.3の6相金属間化合物の水素吸蔵・放出特性を、室温から973 Kの温度範囲、10〜105 Paの水素圧力で研究した。その結果、UZr2.3の水素化によりZrH2およびUH3相への分離が生じた。しかしながら、これらの相の分解等温線はそれぞれの純金属のものとはかなり異なり、この結果は一方の金属元素が他方の金属元素の水素化物相に固溶することに起因すると考えられた。UH3相の形成にもかかわらず、水素化時の合金試料の粉化は著しく低減され、これはおそらくジルコニウムがその中に固溶するためである。したがって、UZr2.3はトリチウムの有望な貯蔵材料であると評価される。

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